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It played a role in promoting aggressive tendencies. (VOY: "The Chute") The reduction acetylcholine levels could help level off neurotransmitter levels and the stabilization of motor neurons. (VOY: "Mortal Coil")
As a choline compound, acetylcholine could be used to stabilize synapses in cases of nervous system collapse. However, it was not effective against the effects of an alien weapon that killed USS Voyager Ensign Ahni Jetal. (VOY: "Latent Image")
An increase of acetylcholine within the hippocampus could indicate that the person had accumulated memories. A thirteen percent increase would indicate an accumulation of two days' worth of memories. (TNG: "All Good Things...")